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Prof. Dr. Uwe Beginn - Publications

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Overview Articles

V. Bakirov, A. N. Yakunin, M. A. Shcherbina, S. N. Chvalun, X. Zhu, U. Beginn, M. Möller, "Ion Channel Forming Self Assembling Systems Based on Benzenesulfonic Acid with Unsaturated Aliphatic Substituents", Nanotechnology in Russia 5(11/12), 762-770 (2010).
U. Beginn, "Polymerization in Supercritical Carbon Dioxide” in “Handbook of Green Chemistry" (P. T. Anastas, ed.), Vol. 4, (Vol. ed.: W. Leitner, P. G. Jessop), pp. 303-368, Wiley-VCH, Weinheim 2010.
U. Beginn, "Gradient Copolymers", Coll. Polym. Sci. 286, 1465-1474 (2008).
U. Beginn, "Continuous Addition Polymerization", e-Polymers, E_003, 1-109 (2005).
U. Beginn, H. Keul, D. Klee, M. Möller, A. Mourran, K. Peter, O. Weichold, "Makromolekulare Chemie 2003", Nachr. Chem. 52, 324 - 331 (2004).
U. Beginn, “Thermotropic columnar mesophases from NH-O, and N-HO hydrogen bond supramolecular mesogenes”, Prog. Polym. Sci. 28, 1049 – 1105 (2003).
U. Beginn, M. Möller, “Supramolecular Structures with Macromolecules“ in “Supramolecular Technology“ (Ed.: D. N. Reinhoudt), Vol. 4, Chap. 3, p. 89 – 176, John Wiley & Sons Ltd., 1999.
U. Beginn, “Supramolecular Templates as Porogenes“, Advanced Materials 10, 1391 - 1394 (1998).
M. Arndt, U. Beginn, T. Heinze, H. Motschmann, "Neue Horizonte in der Polymerforschung" – wissenschaftliches Resümee der Fachgruppentagung Makromolekulare Chemie der GDCh, Mainz, 23.-24. März 1998, Nachrichten aus Chemie, Technik und Laboratorium 46, 1169 - 1171 (1998).

Peer-Reviewed Publications

M. Shcherbina, A. N. Yakunin, U. Beginn, L. Yan, M. Möller, S. N. Chvalun, A. V. Bakirov, "Effect of the Shape of Mesogenic Group on Structure and Phase Behaviour of 2,3,4-tris(dodecyloxy) benzenesulphonates with Alkaline Cations", Soft Matter 10, 1746 – 1757 (2014).

2013
U. Beginn, R. Beckmann, “Synthesis and characterization of new poly(ethyleneimine)-g-poly(methyl methacrylate) star-block copolymers with hyperbranched cationic core“, J. Polym. Sci. A: Polym. Chem. 51(17), 3700-3715 (2013).
U. Beginn, M. Frosinn, M. Reichelt, H. Reuter, “3-Methylideneoxolane-2,5-dione”, Acta Cryst. Sect. E – Structure Reports, E69, o321 (2013).

2012
(a) L. K. Thomas, N. Diek, U. Beginn, M. Reichling, “Dimer/tetramer motifs determine amphiphilic hydrazine fibril structures on graphite“, Beilstein J. Nanotechnol. 3, 658 – 666 (2012).
(b) L. K. Thomas, N. Diek, U. Beginn, M. Reichling, “Dimer/tetramer motifs determine amphiphilic hydrazine fibril structures on graphite“, in “Self-assembly at solid surfaces” (S. R. Cohen, J. Sagiv, eds.), Beilstein J. Nanotechnol., Thematic Series 2012.
S. Asaftei, M. Ciobanu, A. M. Lepadatu, E. Song, U. Beginn, “Thermotropic ionic liquid crystals by molecular-assembly and ion pairing of 4,4’-bipyridinium derivatives and tris(dodecyloxy)benzenesulfonats in a non-polar solvent“, J. Mater. Chem. 22(29), 14426 - 14437 (2012).
M. A. Shcherbina, A. V. Bakirov, A. N. Yakunin, V. Percec, U. Beginn, M. Moeller, S. N. Chvalun, "Self-Assembling Supramolecular Systems of Different Symmetry Formed by Wedged Macromolecular Dendrons", Crystallography Reports 57(2), 151-168 (2012).

2011
U. Beginn, R. Najjar, J. Ellmann, M. Möller, “Polymerization of Vinylidene Difluoride in Supercritical Carbon Dioxide”, Chemie Ingenieur Technik 83, 1419-1442 (2011).
R. Komban, R. Beckmann, S. Rode, S. Ichilmann, A. Kühnle, U. Beginn, M. Haase, “Surface Modification of Luminescent Lanthanide Phosphate Nanorods with Cationic “Quat-Primer” Polymers“, Langmuir 27, 10174–10183 (2011).

2010
L. K. Thomas, A. Kuehnle, S. Rode, U. Beginn, M. Reichling, “Monolayer Structure of Arachidic Acid on Graphite”, J. Phys. Chem. 144, 18919-18924 (2010).
E. Song, J. Podschun, H. Wilberts, U. Beginn, H. Reuter, “Disodium 3,4,5-trihydroxybenzene-1,3-disulfonate dihydrate”, Acta Cryst. E: Struc. Rep. Online E66(10), m1265 (2010).
X. Zhu, A. Mourran, U. Beginn, M. Möller, D. V. Anokhin, D. A. Ivanov, "Self-assembled structures formed by a wedge-shaped molecule in 2D and 3D: the role of flexible side chains and polar head groups", Phys. Chem. Chem. Phys. 12, 1444-1452 (2010).

2008
V. Goel, U. Beginn, A. Mourran, M. Möller, "'Quat-Primer' Polymers bearing cationic and reactive groups: synthesis, characterization and application", Macromolecules 41, 8187-8197 (2008).
U. Beginn, L. Yan, S. N. Chvalun, M. A. Shcherbina, A. Bakirov, M. Möller, "Thermotropic Columnar Mesophases of Wedge-shaped Benzene Sulfonic Acid Mesogens", Liquid Crystals, 35, 1073-1093 (2008).
K. Albrecht, A. Mourran, X. Zhu, T. Markkula, J. Groll, U. Beginn, W. H. de Jeu, M. Möller, "Thin Film Morphologies of Block Copolymers Complexed with Wedge-Shaped Liquid Crystalline Amphiphilic Molecules”, Macromolecules 41, 1728-1738 (2008).

2006
X. Zhu, U. Beginn, M. Moeller, R. I. Gearba, D. V. Anokhin, D. A. Ivanov, "Self-Organization of Polybases Neutralized with Mesogenic Wedge-Shaped Sulfonic Acid Molecules: An Approach toward Supramolecular Cylinders.", J. Amer. Chem. Soc. 128, 16928 – 16937 (2006).
U. Beginn, "Monomer addition programs to generate constant gradient block copolymers", Polymer 47(19), 6880 – 6894 (2006).
X. Zhu, M. A. Scherbina, A. V. Bakirov, B. Gorzolnik, S. N. Chvalun, U. Beginn, M. Moeller, "Methacrylated Self-Organizing 2,3,4-Tris(alkoxy)benzenesulfonate: A New Concept Toward Ion-Selective Membranes", Chemistry of Materials 18(19), 4667 - 4673 (2006).
U. Beginn, R. Najjar, J. Ellmann, R. Vinokur, R. Martin, M. Möller, "Copolymerization of vinylidene difluoride with hexafluoropropene in supercritical carbon dioxide", J. Polym. Sci. A: Polym. Chem. 44(3), 1299 - 1316 (2006).

2005
T. Kitahara, M. Shirakawa, S.-I. Kawano, U. Beginn, N. Fujita, S. Shinkai, "Creation of a Mixed-Valence State from One-Dimensionally Aligned TTF Utilizing the Self-Assembling Nature of a Low Molecular-Weight Gel.", J. Amer. Chem. Soc. 127(43), 14980 – 14981 (2005).
U. Beginn, "COPOINT – a simple computer program to determine copolymerization parameters by numerical integration of copolymerization equations", e-Polymers 073, 1 – 24 (2005).
U. Beginn, L. Yan, X. Zhu, S. Chvalun, M. Möller, "Mimicking Ion Channels by Polymerizable Supramolecular Stacks of Wedge-Shaped Tris(alkenyl-oxy)Benzene Sulfonates", Polymeric Materials: Science & Engineering 93, 244 – 245 (2005).
U. Beginn, S. Weinmann, M. Möller, "Organogels as tool to generate anion : cation selective membranes", Chem. Eng. Commun. 192(8), 1116 - 1128 (2005).
E. Fischer, U. Beginn, N. Fatkullin, R. Kimmich, "Field-gradient NMR diffusometry in poly(ethylene oxide) melts confined to nanoscopic pores of solid methacrylate matrices.", Magnetic Resonance Imaging 23(2), 379-381 (2005).

2004
X. Zhu, B. Tartsch, U. Beginn, M. Möller, "Wedge-Shaped Molecules with a Sulfonate Group at the Tip – A New Class of Self-Assembling Amphiphiles", Chem. Eur. J. 10(16), 3871 - 3878 (2004).
S. Yao, U. Beginn, T. Greß, F. Würthner, "Supramolecular Polymerization and Gel Formation of Bis-Merocyanine Dyes Driven by Dipolar Aggregation", J. Amer. Chem. Soc. 126, 8336 - 8348 (2004).
N. Fatkullin, E. Fischer, C. Mattea, U. Beginn, R. Kimmich,^"Polymer dynamics under nanoscopic constraints: The “corset effect” as revealed by NMR relaxometry and diffusometry", Chem. Phys. Chem. 5, 884 - 894 (2004).
E. Fischer, U. Beginn, N. Fatkullin, R. Kimmich, "Nanoscopic Poly(ethylene oxide) Strands Embedded in Semi-Interpenetrating Methacrylate Networks. Preparation Method and Quantitative Characterization by Field-Gradient NMR Diffusometry", Macromolecules 37(9), 3277 - 3286 (2004).
N. Fatkullin, R. Kimmich, C. Mattea, E. Fischer, U. Beginn, M. Kroutievka, "The confined-to-bulk dynamics transition of polymer melts in nanoscopic pores of solid matrices with varying pore diameter", New J. Phys. 6, 1 - 12 (2004).
A. Mourran, U. Beginn, G. Zipp, M. Möller, "Surface Orientation of 3,4,5-Tris-Substituted Benzoic Acid Amphiphiles", Langmuir 20(3), 673 – 679 (2004).

2003
F. Würthner, S. Yao, U. Beginn, "Highly Ordered Merocyanine Dye Assemblies by Supramolecular Polymerization and Hierarchical Self-Organization", Angew. Chem. Int. Ed. Engl. 42(28), 3247 – 3250 (2003).
U. Beginn, "Applicability of frozen gels from ultra high molecular weight polyethylene and paraffin waxes as shape persistent solid / liquid phase change materials", Macromol. Mater. Eng. 288, 245 – 251 (2003).
U. Haas, C. Thalacker, J. Adams, J. Fuhrmann, S. Riethmüller, U. Beginn, U. Ziener, M. Möller, R. Dobrawa, F. Würthner, “Fabrication and fluorescence properties of perylene bisimide dye aggregates bound to gold surfaces and nanopatterns”, J. Mater. Chem. 13, 767 – 772 (2003).
R. Kimmich, E. Fischer, U. Beginn, N. Fatkullin, A. Denissov, M. Kroutieva, "Polymer chain dynamics in nanopores". Abstracts of Papers, 225th ACS National Meeting, New Orleans, LA, United States, March 23-27, 2003.

2002
H. Götz, U. Beginn, C. F. Bartelink, H. J. M. Grünbauer, M. Möller, "Preparation of Isophorone Diisocyanate Terminated Star Polyethers", Macromol. Mater. Eng. 287, 223 – 230 (2002).

2001
U. Beginn, S. Weinmann, M. Möller, "Organogels as tool to generate anion : cation selective membranes", AIChE Symp. Ser. 153, 406 – 415 (2001).
U. Beginn, B. Tartsch, "Bis[(alkoxy)benzoylsemicarbazides] – a new class of powerful organogelators", Chem. Commun. 2001, 1924 – 1925.
S. Höger, K. Bonrad, A. Mourran, U. Beginn, M. Möller, "Synthesis, Aggregation, and Adsorption Phenomena of Shape persistent Macrocycles with extraannular Polyalkyl Substituents", J. Amer. Chem. Soc. 123, 5651 – 5659 (2001).

2000
S. A. Prokhorova, S. S. Sheiko, A. Mourran, R. Azumi, U. Beginn, G. Zipp, C.-H. Ahn, M. N. Holerca, V. Percec, M. Möller, "Epitaxial Adsorption of Monodendron-Jacketed Linear Polymers on Highly Oriented Pyrolytic Graphite", Langmuir 16, 6862 – 6867 (2000).
U. Beginn, S. S. Sheiko, M. Möller, "Self-Organizing of 3,4,5-Tris(octyloxy)benzamide in Solution and Embedding of the Aggregates into Methacrylate Resins", Macromol. Chem. Phys. 201, 1008 - 1015 (2000).
C. F. Bartelink, M. de Pooter, H. J. M. Grünbauer, U. Beginn, M. Möller, "Controlled formation of isocyanate – terminated star polyethers avoiding chain extension", J. Polym. Sci. A. Polym. Chem. 38, 2555 - 2565 (2000).
U. Beginn, G. Zipp, M. Möller, ‘Synthesis and Characterization of tris-methacrylated 3,4,5-Tris[(alkoxy)benzoyloxy]benzoate derivatives‘, Chem. Europ. J. 6, 2016 – 2023 (2000).
U. Beginn, E. Fischer, T. Pieper, F. Mellinger, R. Kimmich, M. Möller, “Controlled preparation of nanometer sized supramolecular cylinders of poly(ethylene oxide) embedded in methacrylate matrices“, J. Polym. Sci. A: Polym Chem. 38, 2041 – 2056 (2000).
U. Beginn, G. Zipp, A. Mourran, M. Möller, “Membranes Containing Oriented Supramolecular Channels“, Advanced Materials 12, 513 – 516 (2000).
U. Beginn, G. Zipp, M. Möller, “Functional Membranes Containing Ion-Selective ‘Matrix Fixed Supramolecular Channels‘ “, Advanced Materials 12, 510 – 513 (2000).
U. Beginn, G. Zipp, M. Möller, “Self-organization of liquid crystalline methacrylate-trifunctionalized amphiphilic crown-ether derivates in methacrylate mixtures“, J. Polym. Sci. A: Polym. Chem. 38, 631 - 640 (2000).

1999
R. Kimmich, N. Fatkullin, R.-O. Seitter, E. Fischer, U. Beginn, M. Möller, “Intra and Inter-chain Fluctuations in Entangled Polymer Melts in Bulk and Confined to Pore Channels”, Macromol. Symp. 146, 109 – 115 (1999).
R. Kimmich, R.-O. Seitter, U. Beginn, M. Möller, N, Faitkullin, „Field-cycling NMR relaxometry of polymers confined to artificial tubes: verification of the exponent 3/4 in the spin-lattice relaxation dispersion predicted by the reptation model“, Chem. Phys. Lett. 307, 147 – 152 (1999).
E. Fischer, R. Kimmich, U. Beginn, M. Möller, N. Faitkullin “Segment diffusion in polymers confined in nanopores: A fringe field NMR diffusometry study“, Phys. Rev. E. 59, 4079 - 4084 (1999).
S. A. Prokhorova, S. S. Sheiko, A. Mourran, A. E. Semenov, M. Möller, U. Beginn, G. Zipp, C.-H. Ahn, V. Percec, "Epitaxial adsorption of monodendron jacketed linear Polymers on HOPG studied by SFM and STM", Polym. Mat. Sci. Eng. 80, 185 - 186 (1999).

1998
U. Beginn, S. Keinath , M. Möller, "New Carbohydrate Amphiphiles, Part II. Gelation Properties", Macromol. Chem. Phys. 199, 2379 - 2384 (1998).
T. Zavada, S. Stapf, U. Beginn, R. Kimmich, “Field-cycling NMR relaxometry of molecules undergoing Lévy walks at the surface of fine particles and porous glass“, Magnetic Resonance Imaging 16, 711 - 713 (1998).

1997 and before
V. Percec, G. Johansson, G. Zipp, U. Beginn, M. Möller, "Synthesis and characerization of mono-methacrylate functionalized self organizing crown ether compounds", Macromol. Chem. Phys. 198, 265 – 277 (1997).
G. Zipp, U. Beginn, M. Möller, "Self-organization of a liquid crystaline methacrylate-monofunctionalized crown-ether compound in low-shrinkage acrylate mixture", Macromol. Chem. Phys. 198, 2839 - 2852 (1997).
U. Beginn, C. Drohmann, M. Möller, "Conversion Dependence of the Branching Density for the Polycondenzation of AB_n monomers", Macromolecules 30, 4112 – 4116 (1997).
U. Beginn, S. Keinath , M. Möller, "New Carbohydrate Amphiphiles, Part I. Synthesis", Liquid Crystals 23, 35 - 41 (1997).
U. Beginn, G. Lattermann, R. Festag, J. H. Wendorff, "Mesogenic Low and Polymeric Hydrazides, Part II: Mesophase Characterization", Acta Polymerica 47, 214 - 218 (1996).
U. Beginn, G. Lattermann, "Mesogenic Low and Polymeric Hydrazides, Part I: Synthesis", Macromol. Rep. A32(7), 985 - 997 (1995).
U. Beginn, G. Lattermann, "Liquid Crystalline Primary Benzamides", Mol. Cryst. Liq. Cryst. 241, 215 - 219 (1994).

Other Publications

M. J. Kettel, K. Schaefer, A. Koerner, U. Beginn, M. Möller, “Complexation of Synthetic and Natural Insecticides by Cyclodextrines for Both Safe Application and Controlled Release”, Proceedings of the 12^th International Wool Research Conference, ed. Donghua University, Shanghai, P.R. China, Vol. I, Oct. 19-22, 2010, Shanghai / China, pp. 198 – 202.
K. Schaefer, N. V. Belov, U. Beginn, M. Möller, “Nano-coating as Anti-soil Finishes for Textile Floorings”, Proceedings of the 12^th International Wool Research Conference, ed. Donghua University, Shanghai, P.R. China, Vol. I, Oct. 19-22, 2010, Shanghai / China, pp. 203 – 207.
N. Belov, U.Beginn, K. Schaefer, M. Möller, “Synthesis of anhydride reactive fluorinated copolymers and their application for fabrication of superhydrophobic oleophobic surfaces from environmentally fiendly solvents”, Ed. B. Kueppers, Proceedings of the Aachen-Dresden International Textile Conference, 3rd, Aachen, Germany, Nov. 26-27, 2009 (2009).
M. Yu, V. Goel, H. Thomas, U. Beginn, M. Moeller, “Selective surface modification and characterizations of linear and branched polyelectrolyte derivatives”, Proc. Aachen-Dresden Intern. Textile Conf. 2008, MIRA 1 – 10, Dresden, Germany, Dec. 4-5, 2008.
K. Landfester, U. Ziener, M. Möller, U. Beginn, M. Ballauff, "Synthesis of Functional Anorganic Nanoparticles in Supercritical CO₂" in: "Nanotechnology - Physics, Chemistry, and Biology of Functional Nanostructures", (Th. Schimmel, H. v. Löhneysen, Ch. Obermair, M. Barczewski, eds.), Schriftenreihe der LANDESSTIFTUNG Baden-Württemberg, Bd. 32, Stuttgart 2008.
N. Belov, M. Szkudlarek, K. Schaefer, U. Beginn, M. Moeller, "Alternating anhydride-reactive copolymers with perfluorinated side chains for anti-soil textile coatings (AiF 15128 N) ". Proc. Aachen-Dresden Intern. Textile Conf. 2007, 421-430 (2007).
K. Schäfer, U. Beginn, R. Vinokur, A. Giehl, M. Möller, "Extraction with carbon dioxide for removal of contaminants from textiles and materials", Textilveredlung 42, 19-20, 22-24 (2007).
K. Schäfer, U. Beginn, A. Schnurfeil, R. Vinokur, M. Möller , "Purification of textiles and material by extraction with supercritical carbon dioxide (BMBF 01RC0118) ", DWI Reports 2006, 130.
K. Albrecht, A. Mourran, X. Zhu, R. I. Gearba, J. Groll, T. Markkula, U. Beginn, W. H. de Jeu, D. A. Ivanov, M. Moeller, "Supramolecular approach to hierarchical structures in thin films of block copolymers complexed with liquid crystalline amphiphilic molecules", PMSE Preprints 95, 475 – 476 (2006).
M. Moeller, X. Zhu, K. Albrecht, U. Beginn, A. Mourran, M. O. Gallyamov, R. I. Gearba, D. I. Ivanov, "Supramolecular self-organization of polybases complexed with wedge-shaped sulfonic acid molecules". PMSE Preprints 94, 199 (2006).
O. Weichold, X. Zhu, U. Beginn, V. Percec, M. Möller, "Polyelectrolyte-Dendron Complexes: A Route to Template Polymers", Polymeric Materials: Science and Engineering 91, 202 (2004).
R. Kimmich, N. Fatkullin, E. Fischer, C. Mattea, U. Beginn, "Reptation in Artificial Tubes and the Corset Effect of Confined Polymer Dynamics", MRS Proceedings 790, 107 - 118 (2004).
E. Fischer, U. Beginn, A. Denissov, M. Kroutieva, N. Fatkullin, R. Kimmich, "NMR diffusometry on poly(ethylene oxide) confined to nanoporous methacrylate matrices", Polymer Preprints (American Chemical Society, Division of Polymer Chemistry) 44(1), 295 – 296 (2003).
M. Möller, X. Zhu, U. Beginn, ”Template polymerization of monodendritic monomers.” Abstracts of Papers, 223^rd ACS National Meeting, Orlando, FL, United States, April 7-11, 2002.
U. Beginn, E. Fischer, T. Pieper, F. Mellinger, R. Kimmich, M. Möller, “Controlled preparation of nanometer sized cylinder crystals of poly(ethylene oxide) embedded in methacrylate matrices“, Amer. Chem. Soc. Polym. Prepr. 40, 561- 562 (1999).
U. Beginn, G. Zipp, M. Möller, „Polymerisierbare selbstorganisierende Kronenetherderivate für Matrix-fixierte supramolekulare Transportkanäle“, (Hrsg. W. Michaeli, R. Mülhaupt, M. Möller, H. Riedel), Werkstoffwoche 98 – Bd. VIII: Polymere / Simulation Polymere, S. 71 - 76, Wiley-VCH, Weinheim 1999.
U. Beginn, G. Lattermann, "Supramolecular Mesophases via Hydrogen Bonding in Main Chain Polyhydrazides", Polymer Preprints 37, 70 - 71 (1996).

Patents

Chr. Kirsten, M. Moeller, M. Kraus, O. Lammerschop, W. Wolfgang, U. Beginn, “Copolymers containing fluorine, method for the production and use thereof”, Henkel Kommanditgesellschaft auf Aktien, Germany, PCT Int. Appl. (2003), 100 pp. World Patent, WO 2002-EP11276 20021009. Priority: DE 2001-10150954; DE 2002-10231643.
H. Van Aert, B. Groenendaal, H. Andriessen, M. Möller, U. Beginn, A. Mourran, “Heat-sensitive lithographic printing plate precursor”, AGFA-Gevaert, Belgium, EPC Application 04105542.7-2304, 05.11.2004, U.S. Pat. Publ. (2005), US 20050106501 A1 20050519 AN.
M. Moeller, U. Beginn, H. Keul, H. Thomas, "Method for producing adherent coatings to solid surfaces. " DWI an der RWTH Aachen e.V., Germany, Eur. Pat. Appl. (2006), 20pp., EP 1710282 A1 20061011 Application: EP 2005-7306 20050404.